The reason behind the remarkable properties of High-Entropy Alloys (HEAs) is rooted in the diverse phases and the crystal structures they contain. In the realm of material informatics, employing machine learning (ML) techniques to classify phases and crystal structures of HEAs has gained considerable significance. In this study, we assembled a new collection of 1345 HEAs with varying compositions to predict phases. Within this collection, there were 705 sets of data that were utilized to predict the crystal structures with the help of thermodynamics and electronic configuration. Our study introduces a methodical framework i.e., the Pearson correlation coefficient that helps in selecting the strongly co-related features to increase the prediction accuracy. This study employed five distinct boosting algorithms to predict phases and crystal structures, offering an enhanced guideline for improving the accuracy of these predictions. Among all these algorithms, XGBoost gives the highest accuracy of prediction (94.05%) for phases and LightGBM gives the highest accuracy of prediction of crystal structure of the phases (90.07%). The quantification of the influence exerted by parameters on the model's accuracy was conducted and a new approach was made to elucidate the contribution of individual parameters in the process of phase prediction and crystal structure prediction.
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